Hygroscopic aerosols amplify longwave downward radiation in the Arctic


Contact
marion.maturilli [ at ] awi.de

Abstract

This study investigates the impact of hygroscopic aerosols, such as sea salt and sulfate, on longwave downward radiation in the Arctic. These aerosols absorb atmospheric water vapor, leading to wet growth, increased size, and enhanced longwave downward radiation emission, defined as the aerosol infrared radiation effect. Observations of aerosols, especially their composition, are challenging during the Arctic winter. We use an emission Fourier transform spectrometer to measure aerosol composition. Observations show that the aerosol infrared radiation effect of dry aerosols is limited to about 1.45±2.00 W m−2. Wet growth significantly increases this effect. During winter, at relative humidity levels between 60 % and 80 %, wet aerosols exhibit effects approximately 7 times greater than dry aerosols. When relative humidity exceeds 80 %, the effect can be up to 20 times higher. Sea salt aerosols in Ny-Ålesund demonstrate high effect values, while non-hygroscopic aerosols like black carbon and dust show consistently low values. Reanalysis data indicate increased water vapor and sea salt aerosol optical depth in Ny-Ålesund after 2000, correlating with significant positive temperature anomalies in this area. Moreover, wet aerosols can remain activated even in dry environments, continuously contributing high effects, thereby expanding the area affected by aerosol-induced warming. This warming effect may exacerbate Arctic warming, acting as a positive feedback mechanism.



Item Type
Article
Authors
Divisions
Primary Division
Programs
Primary Topic
Research Networks
Publication Status
Published
Eprint ID
60113
DOI 10.5194/acp-25-3889-2025

Cite as
Ji, D. , Palm, M. , Buschmann, M. , Ebell, K. , Maturilli, M. , Sun, X. and Notholt, J. (2025): Hygroscopic aerosols amplify longwave downward radiation in the Arctic , Atmospheric Chemistry and Physics, 25 (7), pp. 3889-3904 . doi: 10.5194/acp-25-3889-2025


Download
[thumbnail of acp-25-3889-2025.pdf]
Preview
PDF
acp-25-3889-2025.pdf - Other

Download (3MB) | Preview

Share
Add to AnyAdd to TwitterAdd to FacebookAdd to LinkedinAdd to PinterestAdd to Email


Citation

Research Platforms


Actions
Edit Item Edit Item